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% Purpose: Proposal for NSF Arctic Natural Sciences (ANS) Dirty Snow project

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% 2005 NSF Arctic Research Opportunities (ARO):
% NSF 05-618
% Office of Polar Programs (OPP)
% Arctic Sciences Section (ASS)
% Arctic Natural Sciences (ANS) Program
% Program Manager, ANS: Jane V. Dionne ``die-on'', (703) 292-7427, jdionne@nsf.gov
% Deadlines: Full Proposal 20051216
% NSF FastLane Temporary Proposal #635594 PIN czen
% NSF FastLane Proposal #0612954 (refer to as ANS-0612954)
% Total 3-year budget request: $403289
% Project duration: 20060701--20090630
% Annual progress report deadlines: 
% Procurement control number (PCN): 
% UCI account number: 9-number-fund-sub-object = 9-123456-12345-1-1234 = 9-445925-12345-1-1234 
% Physical Sciences budget code: 1234

% 2006 NSF OPP ARO ANS Round2:
% Due November 10, 2006

% Usage: See end of file

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% Arctic Natural Sciences (ANS)
\def\prpttl{Dirty Snow on Land, Glaciers, and Sea-Ice: Understanding
 Arctic Absorbing Aerosol Forcing and Feedbacks\\}  
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{\noindent%
On the Web at \url{http://dust.ess.uci.edu/prp/prp_ans-1.0/prp_ans.pdf}\\
NSF Arctic Natural Sciences (ANS) Proposal \hfill Submitted: December~22, 2005\\
Last modified: \today, \xxivtime \hfill Next Round Due: November~10, 2006}
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\textbf{\Large\prpttl}
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Dr. Charles S. Zender \hfill \\
Department of Earth System Science \hfill \\
University of California, Irvine \hfill \\
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\noindent\textbf{News/Preface:} This is NSF proposal 0612954.

\noindent\textbf{Information for potential collaborators:}
This NSF proposal responds to the 2005 NSF Arctic Research
Opportunities (ARO) announcement, NSF 05-618. 
The proposale was submitted to the 
Arctic Natural Sciences (ANS) Program of the
Arctic Sciences Section (ASS) in the
Office of Polar Programs (OPP).
The cognizant Program Manager is Jane V. Dionne \url{jdionne@nsf.gov},
(703)~292-7427.  

Suggestions for next round:
\begin{enumerate}
\item Don't write it in an all-nighter three days before Christmas
\item Make satellite section less cheesey for NASA---e.g., include
  AMSR-E comparison
\item Contact Dorothy Koch for NASA-GISS snow physics collaboration?
\end{enumerate}

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Dr. Charles S. Zender \hfill \\
Department of Earth System Science, University of California, Irvine \hfill \\
\end{center}

\noindent{\large{\textbf{Project Summary.}}}\label{sxn:smr}
%\enlargethispage*{0.5in}

Surface and atmospheric concentrations of black carbon (BC), i.e,
absorbing carbonaceous aerosol, are highly variable and slowly
increasing in the Arctic.  
Current understanding Arctic BC climate impacts derives mostly from
studies which focus on BC direct atmospheric radiative forcing and
which neglect or drastically simplify surface BC interactions. 
However, the prevalence of bright surfaces (snow, glaciers, sea-ice,
and clouds) make the Arctic uniquely susceptible to radiatively
induced effects of surface BC and dust such as ice-albedo feedback
amplification.   
Dirty snow feedbacks change throughout the aerosol lifecycle in the
complex Arctic environment of snowfall, snowpack aging, snow-melt,
drainage, and analogous sea-ice processes.
Our goal is to assess absorbing aerosol interactions in the coupled
Arctic climate system using models which represent the complex surface
lifecycles of Arctic snow, BC, and dust, and which have been evaluated
against satellite, in-situ, and laboratory measurements.  

The project builds upon, extends, and applies our existing,
SNow, ICe, and Aerosol Radiative model, SNICAR.
SNICAR has already helped us show that snowpack aging processes can 
trigger ice-albedo feedbacks which amplify direct surface forcing
by an order of magnitude in mid-latitude regions.
We hypothesize that Arctic BC and dust cause similar, or possibly
greater, ice-albedo feedback amplification over glaciers and sea-ice.
However, current coupled model systems cannot test this hypothesis.
Hence, our project integrates BC, dust and snow lifecycles within 
SNICAR, and places SNICAR in existing coupled snow, ice sheet, and sea
ice models. 

NASA MODIS, MISR, and AMSR-E retrievals will help us constrain model 
parameters, evaluate predictions, and interpret the regional and
seasonal behavior of snowpack processes.
We will support the IPY POLARCAT project by modeling Arctic soot
concentration and snow reflectance following boreal fires.
Snowpack specific surface area, albedo, crystal density,
BC concentration, BC melt scavenging, and aging processes  
will (continue to) be evaluated against Arctic \textit{in~situ}
measurements.  

\textbf{Scientific Merit:}
Our studies of Arctic snow-ice-aerosol processes will improve
understanding of ice-albedo feedbacks and polar climate amplification.  
Key scientific questions we will address include:
1)~Potential for Arctic BC to disrupt summertime sea-ice formation; 
2)~Role of Boreal fire variability in Arctic reflectance, particularly
Greenland; 
3)~Relative roles of Arctic soot and dust in inducing surface melt,
heating, and darkening. 
These questions will be addressed in the context of pre-industrial,
present day, and next century timescales.

\textbf{Broader Impacts:}
Snow pervades the Arctic, and our improved snowpack model can and 
probably will improve understanding of Arctic hydrology.
SNICAR will be freely available to run in both off-line and Community
Climate System Model modes.
We anticipate it will contribute to Arctic research areas including 
glacier mass balance, basin and catchment hydrology, sea-ice
lifecycle, paleoclimate sensitivity, and snow chemistry.
This project trains one graduate student in Arctic aerosol-climate
interactions. 
PI Zender will incorporate this Arctic climate change research into
a K--12 teacher training program and into presentations for lifelong
learning students.
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\section{Introduction}\label{sxn:ntr}

Surface and atmospheric concentrations of black carbon (BC), i.e,
absorbing carbonaceous aerosol, are highly variable and slowly
increasing in the Arctic \cite[][]{PAA01}.  
Current understanding of Arctic BC climate impacts derives mostly
from studies which focus on BC direct atmospheric radiative forcing
and which neglect or drastically simplify surface BC interactions.  
However, bright surfaces (snow, glaciers, sea-ice, and clouds) make
the Arctic uniquely susceptible to radiatively induced effects of
surface BC and dust such as ice-albedo feedback amplification.
Such feedbacks make dirty snow more efficacious than greenhouse gases
at atmospheric temperature change \cite[][]{HaN04}.  
Dirty snow feedbacks change throughout the aerosol lifecycle in the
complex Arctic environment of snowfall, snowpack aging, snow-melt,
drainage, and analogous sea-ice processes
\cite[e.g.,][]{LEM98,AHH03,FlZ06}.   
Our goal is to assess absorbing aerosol interactions in the coupled
Arctic climate system using models which represent the complex surface
lifecycles of Arctic snow, BC, and dust, and which have been evaluated
against satellite, in-situ, and laboratory measurements.  

We use the terms soot and BC interchangeably to denote the light
absorbing component of carbonaceous aerosol \cite[][]{BoB05}.
Interest in BC effects on climate, particularly Arctic climate, has
increased as general circulation model (GCM) aerosol capabilities and
emission inventories have improved.  
Recent noteworthy studies suggest that anthropogenic soot may have
caused one quarter of last century's observed warming
\cite[][]{HaN04}, and significant reductions in Northern hemisphere
albedo and sea-ice extent \cite[][]{Jac04}. 
A lesson learned from our mid-latitude snow studies is that such
estimates are extremely sensitive to accurate treatment of snowpack
aging and radiative transfer \cite[][]{FlZ05}, two areas where this
project will devote significant attention.

Dust can also play an important role in the Arctic, far from its
dominant sources in the sub-tropical deserts \cite[][]{PGT02,ZBN03}.
Dust embedded in Arctic ice cores records global climate change 
\cite[e.g.,][]{AAG98,RaK97,FWJ99,KoH01} and marks periods of abrupt
climate change \cite[e.g.,][]{All00}.
The extent to which this embedded dust may change Arctic and global
climate is still uncertain, and potentially significant for
understanding abrupt climate change mechanisms
\cite[][]{AWL00,HKR01,MML06}. 

Ice-albedo feedback is arguably the most important positive feedback
in the polar climate system \cite[e.g.,][]{Har94,HoB03,QuH06}.
However, we are unaware of any fully interactive
atmosphere-land-ocean-glacier-sea-ice model which accounts for soot
and dust radiative interactions in the surface Arctic.  
Fortunately the necessary component models for an integrated model 
to assess, predict, and improve understanding of Arctic absorbing
aerosol exist \cite[e.g.,][]{CBB06}.
Coupled component models are commonly used to study Arctic climate 
\cite[e.g.,][]{HoB03,HBH06}. 
This project uses high quality component models with realistic
snow-ice-aerosol physics \cite[][]{FlZ05,FlZ06} to ask questions about
the integrated impacts of absorbing aerosols on Arctic climate. 

\csznote{
\begin{enumerate*}
\item Interpreting historical changes in sea-ice extent and fraction
\item Potential for Arctic BC to disrupt summertime sea-ice formation
\item Role of extreme Boreal fire years in Arctic reflectance
\item Use coordinated suite of NASA measurements
\begin{enumerate*}
\item MODIS
\item MISR
\item AMSR-E
\end{enumerate*}
\end{enumerate*}
} % end csznote

% Dusty snowpacks provide additional meltwater on Earth and
% probably other planets \cite[e.g.,]{Clo87}

\subsection{Organization}\label{sxn:org}
This proposal is organized as follows.
Section~\ref{sxn:prr} describes the results of our relevant, prior
NSF-funded research.
The project's historical and scientific context is in
Section~\ref{sxn:bgr}. 
Our scientific objectives and specific hypotheses are in
Section~\ref{sxn:obj}.
Section~\ref{sxn:mth} describes the models and observations we will
use to reach these goals.
Section~\ref{sxn:crd} summarizes the project plan, personnel
responsibilities, time-line, milestones, and travel.
Projects related to ours, potential broader scientific impacts, and
our education plan are in Section~\ref{sxn:mpc}.
Four letters of support/collaboration and a list of acronyms and
abbreviations appear as supplementary documents. 

\section{Results from Prior NSF Funding on Related Projects}\label{sxn:prr}

PI Zender is PI on 
\href{http://www.nsf.gov/awardsearch/showAward.do?AwardNumber=0321380}{ATM-0321380}:
``Acquisition of an Earth System Modeling Facility (ESMF)
for Coupled Climate, Chemistry, and Biogeochemistry Studies''.  
The \href{http://www.ess.uci.edu/esmf}{ESMF} opened in February 2004
and supports about thirty users. 
The ESMF is the main computational resource for UCI's Earth System
Science (ESS) Department.
All ESS modeling groups use the ESMF.
This includes eight professors, four full-time researchers, and about
a dozen graduate students performing global modeling/analysis as part
of their dissertations. 
In order to utilize spare cycles when ESS jobs are not running, 
the ESMF provides free (but lower priority) access to 
researchers/students from any UCI department. 
A summary of (about one dozen) published and in-press papers which
used and acknowledged the collaborative ESMF scientific computing
facility is maintained 
\href{http://dust.ess.uci.edu/prp/prp_mri/prp_mri_apr_02.txt}{here}.

Zender is/was PI on 
\href{http://www.nsf.gov/awardsearch/showAward.do?AwardNumber=0503148}{ATM-0503148}:
``SGER: Improving CCSM Snow/Ice Radiative and Heating Processes and
Assessing the Importance of the Soot Albedo Effect''.
This SGER grant funded graduate student Mark Flanner for one year,
during which he published one paper \cite[]{FlZ05}, placed one
manuscript in review \cite[]{FlZ06}, and gave three national meeting 
presentations.  
\cite{FlZ05} shows that resolving the vertical distribution of solar
radiant heating within snowpack remediates significant climatological
biases in the Tibetan Plateau region.
\cite{FlZ06} study snowpack aging and its effect on albedo.
This the first theoretical study to quantify the relative roles of
initial size distribution, vertical temperature gradient, and snow
density in snow albedo evolution (discussed further in
Section~\ref{sxn:snicar}). 
This proposal requests one year of postdoctoral funding for Flanner.

\section{Background}\label{sxn:bgr}

\subsection{Relevance and Historic Trends}\label{sxn:hst}

Bright surfaces (snow, glaciers, sea-ice and clouds) make the Arctic
uniquely susceptible to radiatively induced effects of surface BC and 
dust such as ice-albedo feedback amplification
\cite[e.g.,][]{HoB03,HaN04,QuH06} (Figure~\ref{fgr:sot_snw_fdb}).  
\begin{figure}
\centering % \centering uses less vertical space than center-environment
\includegraphics[width=0.50\hsize,angle=0,clip=true,trim=1.0in 1.0in 1.0in 1.0in]{/data/zender/fgr/snicar/sot_snw_fdb}%
\caption[Snow-albedo feedback schematic]{
Absorbing aerosols like soot and dust mediate snow-albedo feedback via
multiple paths.  
\label{fgr:sot_snw_fdb}}
\end{figure}
Snow-albedo feedback is triggered by any forcing mechanism which
changes the areal extent of snow cover.
A weaker, positive feedback associated with changes in net surface
radiation is the change in growth rate of snow grains.
Soot in the snowpack directly lowers snow albedo and increases the
growth rate of snow grains, lowering albedo of the ice grains themselves.  
Furthermore, the instantaneous perturbation of soot is greater in
larger-grained snowpack, effectively increasing the gain ($\GGG$) on 
feedback involving grain growth.
Finally, a fourth mechanism perturbation may result from accumulation
of hydrophobic impurities at the surface during melt events, as
supported by observations from \cite{ClN85} and \cite{CGR96}.
Absorbing aerosol also alters cloud reflectivity and lifecycle  
\cite[][]{CLV96,ATS00}.
However, cloud-aerosol effects are not a focus of this project and
will not be further mentioned.

Surface and atmospheric concentrations of black carbon (BC), i.e,
absorbing carbonaceous aerosol, are highly variable and slowly
increasing in the Arctic.
Most emission scenarios project an increase in anthropogenic BC
emissions of 30--250\% in the 21st century
\cite[][]{NAD00,KoH05}.
Changes in fire regime also affect total BC emissions
\cite[][]{VRC04}.
Hence BC impacts on the Arctic will likely increase through the 21st   
century. 

Dust plays an important role in accelerating snow melt in some
mid-latitude regions (Dr.~Tom Painter, NSIDC, personal communication).
Dust-snow interactions may play a very important role in glacial
climates due to increased aridity, equator-to-pole temperature
gradients, exposed continental shelves, and peri-glacial dust
generation \cite[][]{RSK97,MML05,MML06}.
Estimates of past and future dust emissions contain large
uncertainties including those due to land use change and to \COd\
fertilization of vegetative cover \cite[e.g.,][]{MaL03,TWH04}.

Arctic atmospheric and snowpack BC measurements 
span a wide range of concentrations \cite[][]{ClN85,NoC88,HaN04}.
Greenland concentrations are typically 1--4\,\ugxkg, and as high
as 30\,\ugxkg\ \cite[][]{SCD02}.  
Models driven by satellite-derived emissions estimates suggest that
boreal fires explain the largest component of interannual Arctic BC 
deposition variability \cite[][]{KoH05}. 
Our model \cite[][]{FZR05} uses prescribed fossil and biofuel BC
emissions \cite[][]{BSY04}, and converts fire emissions
\cite[][]{VRC03,VRC04,RVC05} to BC with estimated emissions factors 
\cite[]{AnM01}.  
We estimate that biomass burning BC emissions north of 40\dgrn\
increased from 0.1\,Tg to 0.58\,Tg between 1997, a weak fire
year, and 1998, a strong fire year.

We study Arctic climate-aerosol interactions within a coupled general
circulation model (GCM) framework (Section~\ref{sxn:mdl}). 
Using this tool, we estimate Boreal fire emissions changes from 1997
to 1998 increase surface snowpack radiative forcing in the Arctic by
about~50\% \cite[][]{FZR05} (Figure~\ref{fgr:frc_sfc}). 
\begin{figure}
\centering % \centering uses less vertical space than center-environment
\includegraphics[width=0.4\hsize,angle=270,clip=true,trim=0.0in 0.0in 0.0in 1.5in]{/data/zender/fgr/snicar/sotfrc_sfc_1997f11_JJA}%
\includegraphics[width=0.4\hsize,angle=270,clip=true,trim=0.0in 0.0in 0.0in 0.0in]{/data/zender/fgr/snicar/sotfrc_sfc_1998f11_JJA}%
\caption[Snowpack soot direct radiative forcing]{
Summertime mean surface direct radiative forcing [\wxmS] by soot in
snowpack during weak (1997) and strong (1998) boreal burn years.
\label{fgr:frc_sfc}}
\end{figure}
These estimates contain many uncertainties and potential Arctic
aerosol-related biases including transport and deposition, size
distribution, optical properties, aging, and cloud interactions. 
These longstanding issues are targets of ongoing research and
International Polar Year (IPY) activities such as POLARCAT
(Section~\ref{sxn:polarcat}).
More to the point, recent investigations by us and others suggest that 
aerosol-snow interactions play a significant role in Arctic climate
sensitivity via snow-ice-albedo feedback mechanisms on which rapid
progress can be made.

\subsection{Absorbing Arctic Aerosol in Models}\label{sxn:mdl}
The fundamental physics of snowpack-aerosol radiative interactions
have been understood for over 25~years \cite[][]{WiW80,WaW80,Clo87}.
However, few GCMs explicitly account for these effects so the
potentially important polar climate amplification of dirty snow is
largely unstudied.
Models which do not explicitly account for absorbing aerosol may
prescribe snowpack darkening as a function of time since last snowfall
\cite[e.g.,][]{ODB04}. 
This approach is consistent with observations that snowpacks darken
with time due to decreasing snow grain specific surface area (SSA) and 
to increasing impurity concentration (e.g., BC deposition) 
\cite[e.g.,][]{WaW80,AHH03} (Figure~\ref{fgr:niwot}).
\begin{figure}
\centering % \centering uses less vertical space than center-environment
% Rotate Mark's image by 270 degrees so baselines agree
% cd ~/ppr_FlZ06;fl_foo='lggnx';cat ${fl_foo}.eps | epsffit -r 0 0 282 1020 | epsffit -r 0 0 282 1020 | epsffit -r 0 0 282 1020 > ${fl_foo}_270.eps
\includegraphics[width=0.50\hsize,angle=0,clip=true,trim=0.0in 0.0in 0.0in 0.0in]{/home/zender/ppr_FlZ06/fgr_niwot2}%
\includegraphics[width=0.50\hsize,angle=0,clip=true,trim=1.30in 0.0in 1.30in 0.0in]{/home/zender/ppr_FlZ06/lggnx_270}%
\caption[Niwot Ridge albedo decay, Isothermal specific surface area]{
Left Panel: Observed and modeled albedo decay at Niwot Ridge
following the January~2, 2001 snowfall event.
Error bars represent on standard deviation of all measurements
comprising each day's albedo change.
Right Panel: Observed and modeled (SNICAR) isothermal snowpack
specific surface area (SSA) \cite[]{LTD04,FlZ06}.
\label{fgr:niwot}}
\end{figure}
The observed 0.05 snowpack albedo change within four days at Niwot
Ridge illustrates the important role of snowpack aging in controlling
surface energy budgets. 
Prescribed snowpack aging can capture this aging effect on timescales
of a few days.
More sophisticated physics are required to represent longer timescale
albedo evolution \cite[][]{FlZ06}. 

Single layer models are significantly limited in their representation
of aerosol transport and removal mechanisms and in correctly
representing sub-surface radiative heating and melt.
\cite{FlZ05} studied the vertical distribution of solar radiant
heating on snowpack.  
Using accurate radiative transfer methods in a multi-layer snowpack
model (Section~\ref{sxn:snicar}), we showed that 20--40\% of solar
heating occurs beneath the top 2\,\cm\ of typical snowpack.
This sub-surface heating leads to internal snowpack melt.
Internal snowpack absorption can melt snow more efficiently per unit
absorption than surface snowpack absorption which, in the Arctic,
is typically balanced by strong sensible heat fluxes due to cold
overlying air \cite[]{MPB04,FlZ05}.
Snow insulation keeps the internal snowpack warmer than the surface
so that radiatively-induced internal warming can trigger the moderate
snow-grain size-feedback loop (Figure~\ref{fgr:sot_snw_fdb}) until 
melting triggers the stronger snow-cover feedback loop.
%However, all GCMs because they confine solar absorption to the top
%snow layer.   

Today's most sophisticated snow and ice models include Arctic
soot, and, less frequently, dust \cite[][]{Jac04,HaN04,FZR05}.
Interestingly, our preliminary simulations of Greenland show that soot
can reduce total snow melt. 
Significant soot concentrations in the surface snowpack strongly
absorb visible radiation some of which would otherwise penetrate 
into the snowpack (Figure~\ref{fgr:rfl_spc_rds_ffc}). 
\begin{figure}
\centering % \centering uses less vertical space than center-environment
\includegraphics[width=0.50\hsize,angle=0,clip=true,trim=0.0in 0.0in 0.0in 0.0in]{/data/zender/fgr/snicar/snw_sot_spectral_rfl}%
% Rotate Mark's image by 270 degrees so baselines agree
% epsffit coordinate arguments are: llx lly urx ury in Postscript units (points)
% (lower-left x, lower-left y, upper-right x, upper-right y)
% cd ${DATA}/fgr/snicar;fl_foo='rdsffc_1997f11-1998b11_JJA';cat ${fl_foo}.eps | epsffit -r 33 141 543 725 | epsffit -r 33 141 543 725 | epsffit -r 33 141 543 725 > ${fl_foo}_270.eps
\includegraphics[width=0.50\hsize,angle=0,clip=true,trim=0.0in 0.0in 0.0in 0.0in]{/data/zender/fgr/snicar/rdsffc_1997f11-1998b11_JJA_270}%
\caption[Spectral reflectance of snow; Response of effective radius]{
Left Panel: Spectral reflectance of pure snow and snow 
externally mixed with 200\,\ugxkg\ BC for different snow size
distributions.  
Vertical lines show positions of MODIS Bands 3, 4, and~5
(left-to-right). 
Right panel: 
Change in summertime-mean effective radius $\rdsffc$\,[\um] of surface  
snowpack layer due to 1998.
Cross-hatching indicates statistically significant changes 
($\cnfstt < 0.05$) relative to simulations without boreal soot
\cite[][]{FZR05}.
\label{fgr:rfl_spc_rds_ffc}}
\end{figure}
Hence surface soot concentrations can cool the lower snowpack much
as atmospheric soot cools the surface by reducing insolation.
The screening effect of surface soot competes with the
temperature-grain-size feedback (Figure~\ref{fgr:sot_snw_fdb}). 
The ramifications of these competing feedbacks for Arctic climate
remain unknown. 
Nevertheless, it is clear that a prognostic approach which
de-convolves SSA and aerosol effects on snowpack aging and heating
is required for Arctic aerosol-climate impact studies such as this
project. 

Previous efforts to understand absorbing aerosol impacts on the Arctic
have made many approximations which disallow some important feedbacks
that occur in Nature. 
This project, in collaboration with others, will result in a more
complex and interactive Arctic system where 
\begin{enumerate*}
\item Prognostic glaciers allow determination of net hydrology
\item Sea-ice is sensitive to surface aerosol radiative effects
\item Snow-ice-aerosol interactions are consistent across the cryosphere 
\item Soot is treated as fractal aggregates not spheres
\item Snowpack aging reproduces observed features
\item Glacial dust and boreal soot sources are accounted for
%  thermodynamic fixed Qflux sea-ice model in
%  slab ocean (lateral heat transport is prescribed)
%\item Externally mixed soot not internally mixed soot
%\item Provide improvement to global uniform snow grain size assumption
%  for future satellite surface reflectance retrievals.
%\item Goal to monitor Arctic soot/dust concentration from satellites
%No one has retrieved this yet
\end{enumerate*}

%Absorbing aerosol species like soot and dust are typically not
%carried as prognostic, radiatively interactive tracers in 
%Arctic sea-ice models.
%The Arctic Ocean Model Intercomparison Project 
%(\href{http://fish.cims.nyu.edu/project_aomip/overview.html}{AOMIP})
% \cite[e.g.,][]{UHM05}.

\section{Scientific Objectives and Hypotheses}\label{sxn:obj}

Our studies of Arctic snow-ice-aerosol processes will improve
understanding of ice-albedo feedbacks and polar climate amplification 
in Nature, and their representations in models. 
Key scientific questions we will address include:
\setcounter{enmrfr}{0} % Reset reference counter for this list
\begin{enumerate}
\item \enmrfrstp \label{idx_obj_sea_ice} 
\textbf{Objective}: Arctic absorbing aerosol impacts on polar climate 
sensitivity mediated by sea-ice\\  
\textbf{Hypothesis}: Arctic BC can significantly disrupt summer
sea-ice formation and extent during strong burn years\\
Multiple lines of evidence support this hypothesis:
First, representation of thin sea-ice amplifies polar climate
sensitivity \cite[][]{HoB03,HBH06}.
Second, internal snowpack heating amplifies mid-latitude climate
sensitivity \cite[][]{FlZ05}.
Third, aging and absorbing aerosol content increase polar climate
sensitivity \cite[][]{Jac04,HaN04,FZR05}. 
Moreover our preliminary investigations with slab ocean models and
simple sea-ice models suggest a summertime Arctic sea-ice response
to boreal soot in strong fire years.
Summertime Arctic sea-ice extent has been declining in recent decades,  
likely related to greenhouse gas-induced warming
\cite[][]{SMS03,SSF05}. 
We will quantify the extent to which snow-aerosol interactions may
contribute to this trend.
Boreal emissions estimates for recent strong fire years
\cite[][]{RVC05} will allow us to search for connections to
recent accelerations in Arctic sea-ice reduction
\cite[g.g.,][]{SSF05}.  

\item \enmrfrstp \label{idx_obj_sot_dst} 
\textbf{Objective}: Quantify relative roles of Arctic soot and dust 
as polar climate amplifiers\\
\textbf{Hypothesis}: Boreal soot amplifies Arctic climate sensitivity
more/less than dust in the present/LGM climate.\\
Soot is approximately an order of magnitude more absorptive than 
dust at solar wavelengths (assuming single scattering albedos of 
0.5 and 0.95 for soot and dust, respectively).
Dust deposition to Greenland in glacial periods is 2--20 times greater
than present day \cite[e.g.,][]{RaK97,MML06}, enough to compete with
BC as a snow-albedo trigger.
However, differences between BC and dust deposition seasonality and
variability will modulate the net solar forcing of these aerosols 
on Arctic surfaces.
Dust of Asian provenance \cite[][]{BGR97} will likely deposit more
continually than North American glacial dust \cite[][]{MML06}.
The springtime maximum Asian dust export \cite[][]{ZBN03} is less
efficacious for Arctic forcing than summertime aerosol events.
How these spatio-temporal deposition patterns affect Arctic climate
sensitivity is nearly completely unexplored.

\item \enmrfrstp \label{idx_obj_grn_rfl} 
\textbf{Objective}: Role of Boreal fire variability in Arctic
reflectance, particularly Greenland\\ 
\textbf{Hypothesis}: BC warms Greenland in strong fire years and
cools Greenland in weak fire years.\\
Atmospheric BC cools the surface by backscattering and absorbing
incident sunlight.
Snowpack~BC heating compounded by snow-albedo feedback can exceed
atmospheric~BC surface cooling in strong fire years \cite[][]{FZR05} 
(Figure~\ref{fgr:mlt_Grn}).   
Ice core analyses (Dr.~Eric Saltzman, UCI, personal communication) 
and model simulations \cite[][]{KoH05,FZR05} agree that boreal fires 
are the primary source of BC deposition to Greenland in strong fire
years.
We will convolve ice core records of historic BC deposition to
Greenland with present day spatially explicit BC emissions data
\cite[][]{RVC05} to study maximum changes in Greenland reflectance and
melt due to boreal BC over the past 1000~years.  
\end{enumerate}

\section{Methods: Arctic Models and Observations}\label{sxn:mth}

It is important to emphasize that this project will not develop
any Arctic climate model components from scratch.
Our intellectual efforts are primarily directed toward uncovering
the influence of previously neglected snow-ice-aerosol interactions
in the Arctic system.
All model development tasks outlined below involve improving physics
in our in-house snow-ice-aerosol model (SNICAR) and/or merging these
physics into high-quality Arctic system component models developed
and maintained at National centers.  

\subsection{Community Climate System Model}\label{sxn:ccsm}
An integrated Earth System Model which fully couples aerosols, snow,
atmosphere, ocean, and land/sea-ice is required to test our hypotheses 
(Section~\ref{sxn:obj}). 
The NCAR CCSM is that model.
CCSM polar climate simulations have been continually evaluated against
meteorological analyses and satellite observations
\cite[e.g.,][]{BrB981,HoB03,HBH06}.

Arctic absorbing aerosols, soot and dust, are primarily emitted from
non-frozen land surfaces at lower latitudes
\cite[e.g.,][]{ZBN03,KoH05}, and, as such, cut across multiple climate 
``spheres'' (biosphere-atmosphere-cryosphere).
The project relies on our continuing external collaborations for
realistic aerosol distributions and simulation codes.
The CCSM BC/OC aerosol transport, deposition, and optics we use come
from long time collaborators Drs.~Phil Rasch and Bill Collins (NCAR)
\cite[][]{CRE01,CRE02}.

Long time collaborator Dr.~Natalie Mahowald (NCAR, see attached letter
of support) studies atmospheric biogeochemistry and
dust-carbon-climate interactions on multiple timescales.  
Mahowald and PI~Zender are primary developers of the Dust Entrainment 
and Deposition (DEAD) mineral dust model
\cite[][]{ZBN03,ZNT03,MLD03}. 
Ice core measurements are consistent with peri-glacial dust production
during glacial periods \cite[][]{MML06}.
Our simulations will account for this glacial dust production using 
the method and model of \cite{MML06}. 

\subsection{SNICAR}\label{sxn:snicar}
The project builds upon, extends, and applies our existing,
state-of-the-art, SNow, ICe, and Aerosol Radiative model, SNICAR
\cite[][]{FlZ05,FlZ06}.
SNICAR treats snowpack radiative transfer, aging, and aerosol 
interactions in a unified manner that allows for realistic 
feedbacks between solar radiation, snowpack temperature gradients,
and aerosol concentration.
The vertically resolved multi-layer radiative transfer component
\cite[][]{WiW80,TMA89} treats snow as a collection of hexagonal
prisms based on the equivalent surface area-to-volume approximation  
\cite[][]{GrW99,NGW03}.
A lookup table (computed off-line) contains Mie parameters (single
scattering albedo, extinction coefficient, and asymmetry parameter)
for any lognormal size distribution of snow.
SNICAR accounts for solar zenith angle, 
direct and diffuse incident radiation, 
bare surface reflectance \cite[][]{DZD03}, and 
vertically-resolved effective radius (\rdsffc),
snow depth, density, and concentrations of absorbing impurities
\cite[][]{WaW80}.  

An off-line version of SNICAR runs at high spectral resolution,
10\,\nm\ resolution in the solar spectrum from 0.3--5.0\,\um\ 
(470 bands). 
This is useful for simulating narrow-band satellite channels
such as MODIS/MISR channels (Figure~\ref{fgr:rfl_spc_rds_ffc}).
For climate simulations, SNICAR runs in a host snowpack model,
typically the Community Land Model (CLM) \cite[][]{DZD03}.
The CLM uses five vertical snowpack layers \cite[]{ODB04} and itself 
runs off-line forced by meteorological analyses or on-line in a GCM. 

We nest CLM/SNICAR in the Community Atmosphere Model (CAM)
\cite[][]{CRB06} with modifications for prognostic soot driven 
by recent fossil fuel and biofuel emissions estimates
\cite[][]{BSY04}, and biomass burning emissions
\cite[][]{VRC03,VRC04,RVC05}.
Our simulations suggest boreal soot causes seasonal net surface solar    
radiation forcings of 0.5--0.75\,\wxmS\ (Figure~\ref{fgr:frc_sfc})
in strong fire years.
These forcings induce feedbacks such as larger snow grain size
(Figure~\ref{fgr:rfl_spc_rds_ffc}) which together increase seasonal
surface absorption by more than 1.5\,\wxmS\ \cite[][]{FZR05}.
Soot-snow feedbacks in strong fire years appear to cause significant
increases in meltwater production in Greenland snowpack
(Figure~\ref{fgr:mlt_Grn}).
\begin{figure}
\centering % \centering uses less vertical space than center-environment
\includegraphics[width=0.33\hsize,angle=270,clip=true,trim=0.5in 1.0in 0.0in 1.75in]{/data/zender/fgr/snicar/qmelt_1997f11-1998b11_JJA_GR}%
\includegraphics[width=0.33\hsize,angle=270,clip=true,trim=0.5in 1.0in 0.0in 1.75in]{/data/zender/fgr/snicar/qmelt_1998f11-1998b11_JJA_GR}%
\includegraphics[width=0.33\hsize,angle=270,clip=true,trim=0.5in 1.0in 0.0in 0.0in]{/data/zender/fgr/snicar/qmelt_1998g11-1998d11_JJA_GR}%
\caption[Snow melt response to snowpack soot]{
Summertime mean change in Greenland snow melt [\mmxday] due to boreal
soot during low (1997, left) and high (1998, middle and right) boreal
burn years.  
Middle panel includes all feedbacks (soot in atmosphere and snowpack), 
while right panel includes atmospheric soot only.
Cross-hatching indicates statistically significant changes 
($\cnfstt < 0.05$) relative to simulations without boreal soot
\cite[][]{FZR05}. 
\label{fgr:mlt_Grn}}
\end{figure}
Note that neglecting soot-snowpack interactions (and accounting only
for atmospheric soot effects) eliminates or reverses the sign of most
of the increased snow melt over Greenland. 
Hence, \textit{significant Arctic change is attributable to
  aerosol-snowpack feedbacks not represented in most GCMs}.
This makes us eagerly anticipate results in year~3 when SNICAR is 
embedded in fully interactive sea-ice and glacier models which
can respond to soot and to glacial dust sources
\cite[][]{MML06}.  

\subsubsection{Snow Aging}\label{sxn:aging}
Existing representation of snow aging in Arctic climate models is
crude and empirical.  
Some models consider the role of temperature in albedo decay
\cite[][]{Jor91,ODB04} though none consider the dominant role of 
temperature gradient (TG), which requires a multi-layer snow model
such as SNICAR. 
High-latitude snowpack can have temperature gradients well in 
excess of 100\,\kxm\ owing to strong radiative cooling at the surface 
during night, and good thermal insulation of deeper snow.
Vapor-density gradients induced by these temperature gradients cause
rapid snow metamorphism \cite[][]{StB97}.
Using first principles, we account for the roles of initial size
distribution, temperature, temperature gradient, snow density, and
inter-particle spacing in the evolution of snow specific surface area 
(SSA) \cite[][]{FlZ06}.
Vapor diffusion from highly-curved surfaces characteristic of fresh, 
dendritic snow plays a smaller, but non-negligible role in grain
growth via the Kelvin Effect in low TG environments
\cite[e.g.,][]{Col80}. 
Recent SEM observations of well-sintered snow support the hypothesis
that grain-boundary diffusion is an important mechanism in sintering
\cite[][]{RoS06}, although the importance of this mechanism has been 
discounted in earlier studies.  

Meltwater flushing is the most important BC removal mechanism,
since preferential gravitational settling only operates on external
mixtures, and is likely extremely slow.
Qualitative observations suggest that BC may become more concentrated
in surface snow during melt events \cite[][]{WaW80,ClN85}.
\cite{CGR96} spread hydrophobic and hydrophilic BC on top of snow,
and noticed that hydrophobic BC remains in surface snow longer,
maintaining lowered albedo for a longer time.
Because of imprecise knowledge of vertical distributions of BC and
meltwater formation in this experiment, we can only deduce that
hydrophilic BC is scavenged about five times more efficiently than 
hydrophobic BC.
Using a simple $\me$-folding removal model with this data,
we estimate lower bounds for scavenging ratios of 0.01 and 0.002 for 
hydrophilic and hydrophobic BC, respectively.
Even greater uncertainty exists for snow processes on sea-ice.
Planned field studies from Warren and Grenfell
(Section~\ref{sxn:insitu}) will help constrain these scavenging
factors, while current studies by Dr.~Tom Painter (NSIDC) will help 
estimate scavenging efficiency for dust.  

In summary, this project will improve representation of these 
snowpack aging processes in SNICAR:
\begin{enumerate*}
\item Sintering and melting/re-freezing in temporal SSA decay.
  Mark Flanner and Dr.~Tom Painter (NSIDC) will collaborate on 
  representing this process which may be very important for surface  
  albedo in low-TG environments
\item Frost deposition that brightens snow surfaces \cite[][]{Pir04}.  
  We will explore means of parameterizing diurnal SSA increases
  due to hoar frost.
\item Meltwater scavenging of soluble and insoluble aerosols
\end{enumerate*}

\subsubsection{Optics}\label{sxn:opt}
Snow and aerosol optical properties link the snowpack microphysical 
properties (aerosol concentration, particle size distributions)
to macroscopic net absorption (Figure~\ref{fgr:frc_sfc}a), 
reflectances (Figures~\ref{fgr:niwot} and~\ref{fgr:rfl_spc_rds_ffc}a),  
and heating rates that drive the snow melt and temperature change
which trigger snow-albedo feedback.
These responses are sensitive to optical property assumptions which
this project will explore and improve, including 
\begin{enumerate*}
\item BC indices of refraction: 
  \cite{BoB05} question the OPAC properties \cite[][]{HKS98}  
  (which we use) and recommend other measurements including
  \cite{ChC90}    
\item BC shape: 
  Treating BC as spheres likely underestimates its single scattering
  albedo relative to more realistic shapes such as fractal aggregates
  \cite[][]{Sor01,BoB05}
\item Aerosol mixing: 
  BC and dust in remote regions such as the Arctic are primary
  deposited via wet scavenging \cite[][]{CCR01,CSK04,ZBN03} and so will
  often be internally mixed within snow grains.
  We will adopt an effective medium approximation
  \cite[e.g.,][]{BoH83} to represent internally mixed aerosols.
  This will increase snowpack absorption relative to our current
  externally mixed assumption.
%\item Darkening by desert and peri-glacial dust sources \cite[][]{MML06}. 
\end{enumerate*}

\subsection{Sea-Ice and Ice Sheets}\label{sxn:cice}
Sea-ice is the fulcrum of ice-albedo feedbacks in the Arctic Ocean.
Drs.~Bill Lipscomb and Elizabeth Hunke of LANL (see attached
letter of support) are the principle developers of the Los Alamos
sea-ice model 
(\href{http://climate.lanl.gov/Models/CICE}{CICE}), a primary
component of the National Center for Atmospheric Research (NCAR)
Community Climate System Model (CCSM). 
The CICE model contains an Ice Thickness Distribution (ITD) which
maintains a half dozen prognostic categories of ice thickness in
each grid cell \cite[][]{HBH06}. 
The thinnest ice category is most susceptible to changes in net solar 
radiation due to snowpack aging and aerosol concentration.

Accounting for impurities in sea-ice is important to accurate
radiative transfer throughout the atmosphere/ice/ocean system
\cite[]{Gre91}. 
Currently, CICE uses a single layer snowpack upper boundary condition
and neither the sea-ice nor the snowpack tracks absorbing impurities
such as soot and dust as prognostic tracers.
A multi-layer snowpack and prognostic aerosol tracer capability will
be in CICE in 2006 (W.~Lipscomb, personal communication). 
Postdoc Mark Flanner will merge SNICAR physics (snow aging, radiative
transfer, snow-aerosol optics) into this CICE configuration.

The resulting CICE simulations will retain soot and dust deposited
directly on bare sea-ice from the atmosphere and from melting snow
cover.
We hope to use sea-ice radiative transfer physics developed by Bruce
Briegleb (NCAR) to account for aerosols embedded in the complex
sea-ice-brine-pond matrix. 
Sea-ice extent and thickness may then respond to the full lifecycle of
Arctic~BC.  
This will be a significant improvement to current models which remove
BC from snow and sea-ice with rather ad~hoc mechanisms to prevent
excessive concentrations from accumulating in multi-year land and 
sea-ice \cite[][]{Jac04,FZR05}.
Residence time estimates for optically active Arctic soot will improve. 
This may play an important role in studies of
Objective~\ref{idx_obj_sea_ice} (Section~\ref{sxn:obj}).

Lipscomb and Hunke are developing an interactive ice sheet component
for the CCSM.
This ice sheet model is based on
\href{http://wiki.nesc.ac.uk/read/glimmer-project}{GLIMMER}
\cite[]{Pay99}. 
The snow and energy balance model which sits atop GLIMMER will be 
based on the Community Land Model (CLM).
Once postdoc Flanner merges the SNICAR snow-aerosol physics into 
LANL's GLIMMER, the CCSM will have a glacier model component sensitive
to realistic snowpack physics and aerosol interactions.
This will complete the integrated treatment of clean and dirty snow in
the cryosphere.

The ice sheet-aerosol component is scheduled for completion in project
year~3 but may lag due to its complexity and resource issues beyond
our control.
In any case, our numerical studies of the coupled Arctic
land-ocean-sea-ice system with fixed ice sheets will proceed apace
toward Objectives~\ref{idx_obj_sea_ice} and~\ref{idx_obj_sot_dst}
(Section~\ref{sxn:obj}). 

\subsection{Numerical Experiment Strategy}\label{sxn:xpt}
Our questions (Section~\ref{sxn:obj}) will be addressed in the context 
of pre-industrial, present day, and next century timescales when
appropriate.  
Natural (i.e., unforced) interannual variability is quite large in
the Arctic climate system \cite[e.g.,][]{BrB982,FWJ99}. 
Boreal fire variability is also quite large \cite[e.g.,][]{RVC05}
and seems to explain most of the variability in Arctic BC deposition
\cite[][]{FZR05}. 
Detecting and assessing the relatively small (though important) signal
of aerosol-induced Arctic change (Figures~\ref{fgr:rfl_spc_rds_ffc}b
and~\ref{fgr:mlt_Grn}) against the noisy background of natural Arctic
variability is difficult. 

We will continue to employ an ensemble-based approach to increase the 
signal/noise ratio.
The ensemble comprises multiple identical numerical experiments with
slightly perturbed initial conditions.
To obtain the climate responses presented in this proposal we 
conducted perennial 1997- and 1998-emissions experiments in separate  
15\,yr. simulations.
We used a Student's $\ttt$-test to quantify statistical significance
of Arctic changes between the two ensembles.
Significant ($\cnfstt < 0.05$) changes appear as cross-hatched regions
in Figures~\ref{fgr:rfl_spc_rds_ffc}b and~\ref{fgr:mlt_Grn}. 

\subsection{Satellite Observations}\label{sxn:stl}
NASA MODIS, MISR, and AMSR-E retrievals can constrain free model
parameters and help us interpret the regional and seasonal behavior of  
snowpack processes.
Figure~\ref{fgr:rfl_spc_rds_ffc}a shows simulated snow spectral
reflectance expected in visible MODIS bands for various grain sizes.
Soot concentration is most apparent in visible channels and
particle sizes information is most distinguishable in the near
infrared (NIR) \cite[][]{PDR03}, e.g., near MODIS channel~5.

Greenland is an ideal location for evaluation of SNICAR from remote
sensing platforms.
Much of the ice sheet enjoys year round sub-freezing temperatures 
which remove the potentially confounding influence of liquid effects.
Since soot concentrations rarely exceed 5\,\ugxkg\ in Greenland, 
surface snowpack effective radius~$\rdsffc$ is the most promising
model parameters to retrieve and constrain.

Remote sensing of snow grain size has been demonstrated with
hyperspectral airborne instruments such as AVIRIS
\cite[][]{PDR03,DoP04}.  
The same principles apply to MODIS and/or MISR radiances.
However, these satellite products currently have problems associated
with large zenith angles and topography.
Once the MODIS/MISR spectral snow reflectance ($\rfl$) products reach
robust operational status, we will use them to evaluate SNICAR
spectral reflectance, and to try to infer~$\rdsffc$ 
(Figures~\ref{fgr:rfl_spc_rds_ffc}a and~b, respectively).
(We will happily provide our predicted~$\rdsffc$ to any retrieval
experts attempting to improve MODIS/MISR surface reflectance). 
In combination with temperature from meteorological analyses,
retrieved~$\rfl$ and/or $\rdsffc$ will be used to evaluate SNICAR's
snow aging physics \cite[][]{FlZ06} which predict significant
temperature dependence for~$\rdsffc$ (Figure~\ref{fgr:niwot}).

AMSR-E retrieves Snow Water Equivalent (SWE) over non-ice surfaces. 
SWE retrievals may provide useful constraints on SNICAR simulations
of continental snowpack.
In particular, we are interested in assessing the influence of 
extreme aerosol events on the duration of snow cover in seasonally
snow covered regions which are most susceptible to snow-albedo
feedback \cite[][]{FlZ05}. 

\subsection{In Situ Observations}\label{sxn:insitu}
Arctic snowpack BC concentration is the key diagnostic which
integrates aerosol source, transport, deposition, and melt processes.
Drs.~Steve Warren (U.~Washington, see attached letter of support), Tom
Grenfell and Tony Clarke (U.~Hawaii) proposed an ARO project ``Black
carbon in Arctic snow and ice, and its effect on surface albedo''
which will measure BC in snow and ice in tundra regions of Alaska,
Canada, and Russia, as well as on the Greenland Ice Sheet and the
Arctic Ocean to update and improve the BC survey that Clarke conducted
in 1983--1984. 
They will (continue) to share their measurements with us,
including, potentially, BC measurements collected at Dr.~Konrad
Steffen's automated meteorological sites in Greenland. 

Warren et~al.\ will also measure/estimate scavenging coefficients for
removal of atmospheric BC by snow and removal of surface BC during
snow melt (Section~\ref{sxn:aging}).
These scavenging coefficients will provide important constraints for BC
scavenging in CCSM and SNICAR, respectively. 
In addition to Warren and Clarke's earlier measurements,
\cite{FlZ06} evaluated SNICAR against \textit{in situ} and laboratory
measurements of snowpack specific surface area, crystal density,
albedo, and curvature- and temperature-gradient growth processes. 
This project will enable us to continue these comparisons as new data
become available.

\subsection{IPY POLARCAT Participation}\label{sxn:polarcat}
We are contributing to the IPY ``POLar study using Aircraft, Remote
sensing, surface measurements and modeling of Climate, chemistry,
Aerosols and Transport'' 
(\href{http://zardoz.nilu.no/~andreas/POLARCAT}{POLARCAT}) 
(see attached letter from IPY program office to POLARCAT PI~Stohl). 
Our contribution is to one of POLARCAT's main themes---the influence
of boreal fire aerosol on Arctic surface properties.
Although many observational aspects of POLARCAT are still pending,
support for regular aerosol observations at Summit, Greenland appear
to be in place.
Commitments for aircraft campaigns extending from boreal forests to
Greenland are likely in summer 2008.
Using modeled/assimilated BC deposition from NCAR collaborator 
and POLARCAT Steering Committee member P.~Rasch, our group will 
estimate surface reflectance changes at Summit from significant boreal  
events upwind, and compare them to in~situ observations.

The most important measurements we need to help reconcile
discrepancies between our SNICAR model and broadband reflectance
measurements are snow accumulation and vertical profiles of aerosol
concentration, and snowpack temperature.  
Spectral reflectivity would be very valuable but is less likely to
be measured.
We will consider investigating other targets of opportunity which 
may arise during POLARCAT as instrument availability and fire events
allow.

\section{Project Coordination}\label{sxn:crd}

\subsection{Personnel}\label{sxn:prs}

PI~Zender will coordinate all project activities.
Zender has extensive experience in global-scale aerosol modeling
and ice cloud physics and radiative transfer.
Zender will use DEAD \cite[][]{ZBN03} embedded in the CCSM/SNICAR 
with peri-glacial sources \cite[][]{MML06} to provide Arctic dust
deposition fields.
In addition, Zender will develop, test, and implement optical property
improvements in SNICAR, including soot fractal aggregates
\cite[][]{Sor01}, improved refractive indices \cite[][]{ChC90}, and
internally mixed dust/soot/snow properties.

Postdoc Mark Flanner (currently UCI graduate student in ESS) 
will merge SNICAR physics into the CICE sea-ice model and into
the CCSM-compatible version of the GLIMMER ice sheet model provided by 
LANL. 
Scientific specialist Dr.~Chao Luo has specialized in atmospheric
dust transport \cite[][]{LMD03,MaL03,LMJ04} and, more recently, 
cryospheric hydrology based on AMSR-E retrievals.
Luo will assist with coupled model simulations and satellite data
analysis. 

Zender will advise an ESS graduate student in Arctic aerosol studies.
We will initially focus on satellite data analysis of Arctic surface
reflectance. 
In the second and third years, we will use satellite products to help
evaluate and constrain SNICAR, as described in Section~\ref{sxn:stl}.

\subsection{Schedule and Milestones}\label{sxn:tm_ln}
\noindent\textbf{Year~1}. \textit{Milestones}: 
1a.~SNICAR interactive with CICE;
1b.~Fractal aggregate soot;
1c.~Snowpack can brighten diurnally\\
\textit{Tasks}:
\begin{enumerate*}
\item Couple SNICAR physics to sea-ice, examine impact on
  summer melt and extent
\item Update soot optical properties to fractal aggregates
\item Represent hoar frost, diamond dust snowpack brightening
\end{enumerate*}
\textit{Travel}:
\begin{enumerate*}
\item Zender and Postdoc Flanner to Boulder (supported by NCAR
  affiliate scientist and visitor funds) to collaborate with Mahowald 
  and Rasch (NCAR) and Painter (NSIDC)
\item Zender and Postdoc Flanner present results at AGU
\end{enumerate*}
\textbf{Year~2}. \textit{Milestones}: 
2a.~Diurnal snowpack $\rfl$ matches observations;
2b.~SNICAR coupled to LANL glacier-model;
2c.~IPY POLARCAT participation\\
\textit{Tasks}:
\begin{enumerate*}
\item Represent sintering, especially in non-TG snowpacks
\item Refine scavenging with Warren et~al.'s Greenland BC measurements;
\item Compare SNICAR predictions with MODIS/MISR-inferred $\rfl$, $\rdsffc$
\item Quantify Arctic sea-ice sensitivity to soot and dust separately and together
\end{enumerate*}
\textit{Travel}:
\begin{enumerate*}
\item Zender to Norway/NILU for IPY POLARCAT team meeting
\item Graduate student to Los Alamos to merge SNICAR into GLIMMER
\item Zender presents results at AGU
\end{enumerate*}
\textbf{Year~3}. \textit{Milestones}: 
3a.~SNICAR fully coupled in land/sea/glaciers;
3b.~POLARCAT event simulation\\
\textit{Tasks}:
\begin{enumerate*}
\item Estimate soot/dust effect on Greenland accumulation/ablation budgets
\item Integrated absorbing aerosol impact on Arctic climate sensitivity
\item Scale fire emissions from Randerson by ice core data (from
  Saltzman and McConnell) to estimate 1000\,year BC impacts on
  Greenland
\end{enumerate*}
\textit{Travel}:
\begin{enumerate*}
\item PI Zender and graduate student present results at AGU
\end{enumerate*}

\section{Related Projects, Broader Impacts and Education}\label{sxn:mpc}

\subsection{Related Projects}\label{sxn:clb}
This project is synergistic with multiple existing and newly-proposed  
projects.
In addition to collaborative exchanges with LANL, NCAR, and
U.~Washington described within the proposal text and endorsed in
attached letters of support, the following projects will benefit from
ours:  
\begin{enumerate*}
\item Drs.~Steve Warren (U.~Washington, see attached letter of
  support and Section~\ref{sxn:insitu}), Tom Grenfell and Tony Clarke
  (U.~Hawaii).
  We will continue to provide Warren's group with BC deposition
  simulations to aid them in choosing BC measurement site locations. 
\item Drs.~Natalie Mahowald (see attached letter of support and
  Section~\ref{sxn:ccsm}) and Phil Rasch (NCAR). 
  We will continue to make SNICAR code improvements available to NCAR
  CCSM component models. 
  Mahowald and Dr. Peter Thornton are investigating changes in boreal
  fire regime in a dynamic vegetation and carbon/nitrogen cycling
  framework. 
  The more realistic lower boundary condition SNICAR provides will
  improve these studies' realism.
\item Drs.~Bill Lipscomb and Elizabeth Hunke, LANL
  (see attached letter of support and Section~\ref{sxn:cice}).
\item Dr.~Tom Painter (NSIDC) studies snow aging, dust-driven
  heating of mid-latitude snowpacks, and retrieval of snowpack
  reflectance, size distribution and impurities from remote sensing
  instruments.
  Painter will use SNICAR physics within the SNTHERM snowpack model to 
  account for dust-snowpack interactions on catchment/basin scale
  hydrology.  
\item Drs.~Jim Randerson and Yufang Jin (UC~Irvine) are our primary 
  in-house collaborators on boreal soot impacts.
  Their integrated studies of C-cycling along boreal fire
  chronosequences provide the fire emissions estimates which drive
  our simulations \cite[e.g.,][]{RVC05}. 
  We will continue to collaborate with them on integrated forcing
  estimates from boreal fires and to use CCSM/SNICAR to quantify soot
  indirect effects such snowpack-mediated radiative forcing
  \cite[][]{FZR05,RLF05}. 
\item Dr.~Eric Saltzman (UC~Irvine) measures trace gas and aerosol 
  concentrations in ice cores \cite[e.g.,][]{SAD04} and Co-PIs a 
  proposed ARO project ``High-Resolution, Biomass-Burning-Specific
  Tracers in Greenland Ice Cores over the Past 1000~Years''.
  In conjunction with Randerson's fire emission database, our project
  provides a method to quantify the impact of Saltzman's proxy
  measurements of biomass burning aerosol variability in Greenland
  over the last 1000\,yr. 
\end{enumerate*}

\subsection{Improved Community Modeling Capabilities}\label{sxn:mdl_mpr}
Snow pervades the Arctic, and improved snowpack models can and
probably will improve understanding of Arctic hydrology.
Zender has provided many useful research models to various communities
including the Column Radiation Model 
(\href{http://www.cgd.ucar.edu/cms/crm}{CRM}),
the Dust Entrainment and Deposition Model
(\href{http://dust.ess.uci.edu/dead}{DEAD}),
and the netCDF Operators (\href{http://nco.sf.net}{NCO}).
SNICAR will be freely available both in off-line and in Community
Climate System Model modes.
We anticipate SNICARS and its physics will contribute to Arctic
research areas including glacier mass balance (through realistic upper
boundary radiation and melt conditions),  
basin and catchment hydrology (improved representation of snowpack
sublimation vs.\ internal melt and surface percolation), 
sea-ice lifecycle (improved upper boundary condition), 
paleoclimate sensitivity (through improved accuracy of Arctic
responsiveness to orbital and aerosol forcing),  
and snow chemistry (through improved representation of snowpack
specific surface area).

\subsection{Education}\label{sxn:edc}
This project trains one graduate student in Arctic aerosol-climate
interactions.
Moreover, PI~Zender helps train Orange County K--12 teachers in Earth
Science curricula. 
An NSF Math Science Partnership project called
\href{http://focus.mspnet.org}{FOCUS}  
(Faculty Outreach Collaborations Uniting Scientists, Students and
Schools)
brings the teachers to UCI.
Zender will incorporate Arctic climate change materials into 
\href{http://dust.ess.uci.edu/smn/smn_sun_focus_200508.pdf}{his FOCUS seminars}.
Zender will also incorporate this Arctic research into his
\href{http://dust.ess.uci.edu/smn/smn_sun_olli_200511.pdf}{seminars}
to students of the Osher Lifelong Learning Institute 
(\href{http://unex.uci.edu/community/olli/index.asp?}{OLLI}).
\newpage

\section*{References}\label{sxn:rfr} % \section* does not number section
\setcounter{page}{1}
\thispagestyle{empty}
% Bibliography
\renewcommand\refname{(blue numbers show proposal section where citation occurs)}
\vspace{-24.0pt}
\newlength{\oldbaselineskip}
\setlength{\oldbaselineskip}{\baselineskip}
%\setlength{\baselineskip}{13.574pt} % 1.234 X 12pt
\setlength{\baselineskip}{12.0pt} % 1.234 X 11pt
\setlength{\bibsep}{4pt} % Space between natbib bibliography items
\bibliographystyle{jas}
\bibliography{bib}
\setlength{\baselineskip}{\oldbaselineskip} % 1.851 X 11pt
\newpage
\printindex % Requires makeidx KoD95 p. 221
\addcontentsline{toc}{section}{Index}
\newpage

\subsection{Budget Justification}\label{sxn:bdg_jst}
\setcounter{page}{1}
\thispagestyle{empty}
\begin{verbatim}
% NB: Do not use LaTeX formatting in Budget Justification since must
% upload into Liz's Word document 

Salaries and Wages

One month of summer salary support for three years is requested for
Prof. Charles Zender, the PI, who has primary responsibility for the
proposed research.  
Salary support for Mark Flanner, a postdoctoral scholar is requested
in year 1. Dr. Flanner is responsible for fully coupling the SNICAR
aerosol/snowpack model to the glacier dynamics model and to the
sea-ice model, and for performing initial fully coupled studies. 

Funds are requested to to support Dr. Chao Luo, Associate Specialist
Step II, at a rate of 0.2 FTE for the duration of the project.
Dr. Luo is the principal scientific programmer associated with 
UCI's Earth System Modeling facility.
Dr. Luo has run the complex models involved in this project (SNICAR,
DEAD, CLM, CAM, CCSM) and will devote 20% of his time to performing
and to analyzing coupled model studies.
A 2% cost of living increase was applied each year of this proposal
as well as a 5% merit, where applicable.

To be Named---Graduate Student Researcher III.  Funds are requested to
support one non-resident graduate student each year of the project.
The graduate student support is requested at 50% for 9 months during
the academic year and 100% for 3 months during the summer. 
The graduate student will work on isolating and evaluating dirty
snowpack signatures in satellite data, modeling soot transport events
in support of IPY POLARCAT, and, in year 3, performing fully coupled
model studies.
All salaries and wages were estimated using UCI's academic and staff
salary scales.  

Employee Benefits
Fringe Benefits were estimated using the composite rates agreed upon
by the University of California Office of the President and the DHHS
Audit Agency, the Cognizant Audit Agency for the University of
California.  Benefit rates used in this proposal are: 
Faculty - summer - 12.7%
Academic (Specialist) - 17%
Student employees - summer - 3%
Student employees - academic year - 1.3%

Fees are requested for one nonresident student for the duration of the
project. University of California policy requires award payment of
fees for any student with more than 25% support from a grant.  In the
first year, $26,690 is requested for non-resident fees and tuition,
$29,258 in the second year. It is anticipated that the graduate
student will advance to candidacy at the beginning of the third year.
University policy provides a 75% reduction in nonresident tuition post
advancement.  Therefore, fees and tuition are reduced to $16,748 in
year 3.  Fees and tuition are excluded from indirect cost assessment.   

Equipment
Equipment funds are requested for the first year only for one dual
Opteron, dual core workstation at $6,000. This workstation will
include adequate RAID'ed disk space (1 TB) for the graduate student
to store and analyze satellite MODIS, MISR, and AMSR-E datasets.

Travel
Domestic:  Round-trip travel at $1500 per trip is requested for the PI
and Postdoc (year 1) or graduate student (years 2 and 3) to travel to
national meetings (primarily AGU) to present results. 
Each trip includes roundtrip travel from Irvine to San Francisco or
the East Coast, one-week hotel and per diem. 
These trips include estimated conference registration, abstract
submission fees, RT airfare, lodging, meals and ground transportation.
Travel estimates are based on historical usage. 

International:  One round-trip at $3000 is requested for the PI to
travel to Norway in Year 2 to participate in the IPY POLARCAT team
meeting activities and to present results. 
This trip includes roundtrip travel from Irvine to Oslo, one-week
hotel and per diem.  
These trips include estimated conference registration, abstract
submission fees, RT airfare, lodging, meals and ground transportation.
Travel estimates are based on historical usage. 

Other Direct Costs
Charges for journals, photocopying, long distance phone, fax and
postage charges pursuant to this project are requested each year.
Included in these expenses are long-distance charges for usage
directly related to the project, such as communication with
colleagues, journals, and vendors.    Photocopying of research
materials including publications and results of this sponsored
research project are requested as well as mail and shipping for
materials related to this project. Support is requested in years 2 and
3 for publication costs pursuant to this project, which include
utilization of expensive color figures.  Costs were estimated
according to historical usage. 

Indirect Costs
Facilities and Administrative costs were estimated in accordance with
UCI's approved indirect cost rate agreement. 
The indirect cost rate of 52.5% of MTDC effective 7/1/05 was based
upon the nature and location of the work proposed.  
Graduate student fees and tuition and equipment are excluded from
indirect cost assessment.  
UCI's indirect cost rate agreement was approved by DHHS,
the Federal Cognizant Audit Agency for UCI on 12/5/01. 
\end{verbatim}
\newpage

\section{Facilities, Equipment, and Other Resources}
\subsection{Computational Resources}
\setcounter{page}{1}
\thispagestyle{empty}
Our ANS project is well-situated to take advantage of UCI's fast
computing capabilities previously funded by NSF and other agencies.

PI~Zender directs the Earth System Modeling Facility (ESMF), 
an NSF-supported MRI facility dedicated to coupled global climate,
chemistry, and biogeochemistry simulations.
The ESMF flagship machines is an 88-CPU Power4+ IBM supercomputer with
192\,\GB\ RAM and 16\,\TB\ of RAID storage.
In Spring 2006, ESMF anticipates acquiring a new Beowulf cluster
comprising approximately twenty two-way dual core Opteron nodes
(80~CPUs) and about 5\,\TB\ of RAID storage.
Since this ANS proposal is squarely fits the ESMF mission, the ESMF
will host the primary modeling development and shorter simulations.
Once this project is funded, we will request supplementary time at
NCAR for long production simulations of the fully coupled CCSM/SNICAR 
code. 
\newpage

\section{Acronyms and Abbreviations}\label{sxn:abb}
\setcounter{page}{1}
\thispagestyle{empty}
%\begin{longtable}{ >{\raggedright}p{7.0em}<{} >{\raggedright}p{8.0em}<{} }
\begin{longtable}{ r >{\raggedright}p{25.0em}<{} l }
& \kill % NB: longtable requires caption as table entry
\caption[Acronyms and Abbreviations]{\textbf{Acronyms and Abbreviations}%
\label{tbl:abb}} \\
\hline\hline \rule{0.0ex}{\hlntblhdrskp}% 
Abbreviation & Description & \\[0.0ex]
\hline \rule{0.0ex}{\hlntblntrskp}%
\endfirsthead % Lines between and \endfirsthead appear at top of table
\caption[]{(continued)} \\ % Set label for following pages
Abbreviation & Description & \\[0.0ex]
\hline \rule{0.0ex}{\hlntblntrskp}%
\endhead % Previous block appears at top of every page
\endlastfoot % Previous block appears at end of table
AAA & Arctic Absorbing Aerosol & \\
AMSR-E & Advanced Microwave Scanning Radiometer (satellite instrument) & \\
ANS & Arctic Natural Sciences & \\
AOMIP & Arctic Ocean Model Intercomparison Project & \\
AR4 & Fourth Assessment Report & \\
ARF & Aerosol Radiative Forcing & \\
ATSR & Along Track Scanning Radiometer and Microwave Sounder & \\
AVIRIS & Airborne Visible/Infrared Imaging Spectrometer & \\
BC & Black Carbon (light-absorbing component of carbonaceous aerosol) & \\
BRDF & Bi-directional Reflectance Distribution Function & \\
CAM & Community Atmosphere Model & \\
CCSM & Community Climate System Model & \\
CFEP & Center for Educational Partnerships & \\
CICE & Los Alamos sea-ice model & \\
CLM & Community Land Model & \\
CRM & Column Radiation Model & \\
DEAD & Dust Entrainment And Deposition Model & \\
EMA & Effective Medium Approximation & \\
ESM & Earth System Model & \\
ESMF & Earth System Modeling Facility & \\
ESS & Earth System Science (Department) & \\
FOCUS & Faculty Outreach Collaborations Uniting Scientists, Students and Schools & \\
GCM & General Circulation Model & \\
GFED & Global Fire Emissions Database & \\
GHG & Greenhouse Gas & \\
GLIDE & General Land Ice Dynamic Elements (core of GLIMMER) & \\
GLIMMER & Ice Sheet Model of Payne et~al. & \\
GSFC & Goddard Space Flight Center & \\
IPCC & Intergovernmental Panel on Climate Change & \\
IPY & International Polar Year & \\
ITD & Ice Thickness Distribution & \\
LANL & Los Alamos National Laboratory & \\
LGM & Last Glacial Maximum & \\
MISR &  Multi-angle Imaging Spectro-Radiometer (satellite instrument) & \\
MODIS &  Moderate Resolution Imaging Spectroradiometer (satellite instrument) & \\
NASA & National Aeronautic and Space Administration & \\
NCAR & National Center for Atmospheric Research & \\
NCO & netCDF Operators & \\
NILU & Norwegian Institute for Air Research & \\
NIR & Near InfraRed & \\
NSIDC & National Snow and Ice Data Center & \\
OC & Organic Carbon & \\
OLLI & Osher Lifelong Learning Institute & \\
OPAC & Optical Properties of Aerosols and Clouds & \\
PI & Principle Investigator & \\
POLARCAT & POLar study using Aircraft, Remote sensing, surface measurements and modeling of Climate, chemistry, Aerosols and Transport (IPY project) & \\
RT & Radiative Transfer & \\
SEI & Science and Engineering Informatics & \\
SEM & Scanning Electron Microscopy & \\
SGER & Small Grant for Exploratory Research & \\
SNICAR & SNow, ICe, and Aerosol Radiative model & \\
SNTHERM & Snow Melt model & \\
SOM & Slab Ocean Model & \\
SSA & Specific Surface Area & \\
SWE & Snow Water Equivalent & \\
TG & Temperature Gradient & \\
UCI & University of California, Irvine & \\
\end{longtable} % end tbl:abb
\newpage

\section{Project-Wide Combined Collaborator and Advisor List}\label{sxn:prs_lst} 
\setcounter{page}{1}
\thispagestyle{empty}
% Currently includes: Zender
All Personnel Associated with Proposal, Collaborators and
Co-Editors of Project Senior Personnel, their Post-docs, and their
Thesis Advisors:
\begin{enumerate*}
\item[] Ammann, C.~A. (NCAR) 
\item[] Bian,~H. (NASA/UMBC) 
\item[] Bonan, G.~B. (NCAR) 
\item[] Busacca,~A. (WSU)
\item[] Cakmur,~R. (NASA GISS) 
\item[] Colarco,~P. (GSFC)
\item[] Collins, W.~D. (NCAR) 
\item[] Cooper, W.~A. (NCAR)
\item[] Famiglietti,~J. (UCI) 
\item[] Gaylord,~D. (WSU)
\item[] Grini,~A. (U.~Oslo)
\item[] Jenks,~S. (UCI) 
\item[] Khalsa, S.~J.~S. (NSIDC)
\item[] Kiehl, J.~T. (NCAR) 
\item[] Kuester,~F. (UCI) 
\item[] Levin,~Z. (TAU, Israel) 
\item[] Mahowald, N.~M. (NCAR) 
\item[] Miller,~R. (NASA GISS) 
\item[] Moore, J.~K. (UCI) 
\item[] Okin,~G. (U.~Virginia) 
\item[] Painter,~T. (NSIDC) 
\item[] Pajarola,~R. (UCI) 
\item[] Papadopoulos,~P. (UCI)
\item[] Rasch, P.~J. (NCAR)
\item[] Tegen,~I. (IfT, Germany) 
\item[] Thomas, G.~T. (CU) 
\item[] Torres,~O. (NASA GSFC)
\item[] Valero, F.~P.~J. (Scripps) 
\item[] Yu,~S. (Duke) 
 \end{enumerate*}
\newpage

List is Alphabetical by Surname.
\begin{enumerate*}
\item[] Collaborators of Zender:
\begin{enumerate*}
\item[] Ammann, C.~A. (NCAR) 
\item[] Bian,~H. (NASA/UMBC) 
\item[] Bonan, G.~B. (NCAR) 
\item[] Busacca,~A. (WSU)
\item[] Cakmur,~R. (NASA GISS) 
\item[] Colarco,~P. (GSFC)
\item[] Collins, W.~D. (NCAR) 
\item[] Cooper, W.~A. (NCAR)
\item[] Famiglietti,~J. (UCI) 
\item[] Gaylord,~D. (WSU)
\item[] Grini,~A. (U.~Oslo)
\item[] Jenks,~S. (UCI) 
\item[] Khalsa, S.~J.~S. (NSIDC)
\item[] Kiehl, J.~T. (NCAR) 
\item[] Kuester,~F. (UCI) 
\item[] Levin,~Z. (TAU, Israel) 
\item[] Mahowald, N.~M. (NCAR) 
\item[] Miller,~R. (NASA GISS) 
\item[] Moore, J.~K. (UCI) 
\item[] Okin,~G. (U.~Virginia) 
\item[] Painter,~T. (NSIDC) 
\item[] Pajarola,~R. (UCI) 
\item[] Papadopoulos,~P. (UCI)
\item[] Rasch, P.~J. (NCAR)
\item[] Tegen,~I. (IfT, Germany) 
\item[] Thomas, G.~T. (CU) 
\item[] Torres,~O. (NASA GSFC)
\item[] Valero, F.~P.~J. (Scripps) 
\item[] Yu,~S. (Duke) 
  \end{enumerate*}
\item[] Collaborators of Co-PI Dr.~Who:
\begin{enumerate*}
\item Hi
\end{enumerate*}
\end{enumerate*}
\newpage

\subsection{Supplementary Documents}\label{sxn:spl_doc}
\setcounter{page}{1}
\thispagestyle{empty}
\begin{verbatim}
1. ${DATA}/prp/prp_ans/prp_ans_ltr_warren.pdf
2. ${DATA}/prp/prp_ans/prp_ans_ltr_lanl.pdf
3. ${DATA}/prp/prp_ans/prp_ans_ltr_mahowald.pdf
4. ${DATA}/prp/prp_ans/prp_ans_ltr_polarcat.pdf
5. ${DATA}/prp/prp_ans/prp_ans_clb.pdf
6. ${DATA}/prp/prp_ans/prp_ans_abb.pdf
\end{verbatim}

\clearpage

\csznote{
% Text snippets for future proposals...
} % end csznote

\csznote{
# Dozier's pubs
http://www.snow.ucsb.edu/REASoN-Publications.htm

# Email distribution list
Siri Jodha Singh Khalsa <sjsk@nsidc.org>,
Tom Painter <tpainter@nsidc.org>,
Jim Randerson <jranders@uci.edu>,
Mark Flanner <mflanner@uci.edu>,
Jorge Talamantes <jtalamantes@csub.edu>,
Charlie Zender <zender@uci.edu>

% Letter sent to Bill Lipscomb 20051215:
Dear Bill,

Thanks for discussing collaborations on the phone yesterday.
As I said, I am following up with a one page summary of our proposed
NSF project, and some sample text should you choose to endorse our
collaboration more formally with NSF. Please feel free to
ruthlessly alter/edit! The below text is meant to save you time, not
to constrain you or to obligate you to do work you're not already
interested in. If you choose to write such a letter, it would be
most helpful if you could e-mail me a PDF on your letterhead by
Wednesday morning 12/21, although a simple e-mail will suffice if you
are too busy for the deluxe PDF option.

Thanks!
Charlie

"Dear Charlie,

As one of the principle developers of the Los Alamos sea-ice model
(CICE), a primary component of the
National Center for Atmospheric Research (NCAR)
Community Climate System Model (CCSM),
I have a great interest in understanding and correctly representing
the coupled cryosphere in Earth System Models.
Your proposed NSF project "Dirty Snow on Land, Glaciers, and Sea-Ice:
Understanding Arctic Absorbing Aerosol Forcing and Feedbacks" would
continue to advance the state-of-the-art in snowpack radiative
transfer which provides an important upper boundary condition in the cryosphere.
We are happy to collaborate with you and Mark Flanner in two related
areas during the NSF project.

First, we are implementing a multi-layer snow thermodynamic model to
improve the current single layer snow model in CICE.
We will provide source code access and advice on technical details
so that your project can merge SNICAR physics for snowpack aging and
radiative processes into CICE.
Second, we are developing an interactive ice sheet component, based
on GLIMMER, for the CCSM.
We envisage using the a form of the Community Land Model (CLM) and its
snow model with SNICAR as the upper boundary condition.
The integrated treatment of clean and dirty snow in the cryosphere
which will result from our complementary efforts will provide a
state-of-the-art toolkit with which to study the scientific questions
posed in your proposal."

% Letter sent to Steve Warren 20051215:
Dear Steve,

As I said, I am following up with some sample text should you choose
to endorse our collaboration more formally with NSF. Please feel free
to ruthlessly alter/edit! The below text is meant to save you time,
not to constrain you or to obligate you to do work you're not already
interested in. If you choose to write such a letter, it would be
most helpful if you could e-mail me a PDF on your letterhead by
Wednesday morning 12/21, although a simple e-mail will suffice if you
are too busy for the deluxe PDF option.

P.S. As I think you already know, SNICAR uses optical properties based
on your and Grenfell's work on the surface-area-to-volume Mie
approximation. Thanks again for developing this useful approximation!

Charlie

"Dear Charlie,

As you know I have a great interest in understanding snow, ice, and
Arctic aerosol properties and I approach these topics from a
combination of laboratory and in situ measurements combined with
radiative transfer modeling.
Your proposed NSF project "Dirty Snow on Land, Glaciers, and Sea-Ice:
Understanding Arctic Absorbing Aerosol Forcing and Feedbacks" would
continue to advance the state-of-the-art in snowpack radiative
transfer which provides an important upper boundary condition in the
cryosphere. Moreover, your coupled snowpack aging and radiation model,
SNICAR, is a very suitable tool for hind-casting the snowpack BC
concentrations in Greenland which our group continues to measure.

Our newly proposed NSF project "title goes here" will fund us to
measure BC from snow samples collected at all Koni Steffen's AWS
sites, which will provide good coverage of the Greenland ice sheet. 
We will be pleased to provide your project with these measurements and
to collaborate on their interpretation.
The synergy between our measurements and your modeling project
to understand and represent Arctic snow-ice-aerosol feedbacks is
exciting."

% Letter sent to Phil Rasch 20051215:
Hi Phil,

We are writing an NSF Arctic proposal called "Dirty Snow on Land,
Glaciers, and Sea-Ice: Understanding Arctic Absorbing Aerosol Forcing
and Feedbacks". The proposal would fund a grad student, and a one year
postdoc which Mark Flanner can use as bridge funding. The goal is
to continue studying dirty snow, both BC and dust, and to move to
the next level of feedbacks by really including sea-ice and glacier
effects. We think we have land pretty well covered, and will work
with Bill Lipscomb (and probably Bruce Briegleb, although I'm a bit
unsure where that stands) on the sea-ice and glacier coupling to
SNICAR.  

Mark is beginning to write a boreal soot manuscript on which you will
be offered co-authorship. Not making you an official co-author on the
study Mark presented at AGU was an oversight! Although we fixed it in
the title slide your name was not in the program. Apologies.

Back to the present. This proposal is due Thursday 12/22 (I got an
extension to improve the collaboratory aspects of the proposal).
This proposal will rely heavily on continued use of your BC aerosol
model in CAM. I am verifying that we can rely on you for this,
and that I can mention this in the proposal's collaborative portion.
Is there anything I should know or that you'd like to add?
Attached is the current one-page summary FYI.

Thanks,
Charlie

% Letter sent to Natalie Mahowald 20051215:
Hi Natalie,

We are writing an NSF Arctic proposal called "Dirty Snow on Land,
Glaciers, and Sea-Ice: Understanding Arctic Absorbing Aerosol Forcing
and Feedbacks". The proposal would fund a grad student, and a one year
postdoc which Mark Flanner can use as bridge funding. The goal is
to continue studying dirty snow, both BC and dust, and to move to
the next level of feedbacks by really including sea-ice and glacier
effects. We think we have dirty land-snow pretty well covered, and
will work with Bill Lipscomb (and probably Bruce Briegleb, although
I'm a bit unsure where that stands) on the sea-ice and glacier
coupling to SNICAR.  

This proposal is due Thursday 12/22 (I got an extension to improve the
collaborative aspects of the proposal). 
This proposal will rely heavily on continued use of Phil's BC aerosol 
model in CAM and on your dust code, if you agree. 
May we rely on you for code access and advice as has been our habit?
It would be especially cool to include your glaciogenic dust sources
(pun intended). Of course, we'll offer you co-authorship on any of the
dust-related results. 
If you agree, may I mention this in the proposal's collaborative portion?
Is there anything I should know or that you'd like to add?
Attached is the current one-page summary FYI.

Thanks,
Charlie
} % end csznote

\csznote{
% Usage: Place usage here at end of file so comment character % not needed
cd ~/prp_ans-1.0;make -W prp_ans.tex prp_ans.dvi prp_ans.ps prp_ans.pdf prp_ans.txt;cd -
scp ${HOME}/prp_ans-1.0/prp_ans.dvi ${DATA}/ps/prp_ans.pdf ${DATA}/ps/prp_ans.ps ${HOME}/prp_ans-1.0/prp_ans.tex ${HOME}/prp_ans-1.0/prp_ans.txt dust.ess.uci.edu:/var/www/html/prp/prp_ans-1.0
scp ${DATA}/ps/bio_nsf.pdf ${DATA}/prp/prp_ans/prp_ans_cv_zender.pdf

# NB: latex2html works well on prp_ans.tex
latex2html -dir /var/www/html/prp/prp_ans prp_ans.tex
# NB: tth chokes on prp_ans.tex
cd ${HOME}/prp_ans-1.0;tth -a -Lprp_ans -p./:${TEXINPUTS}:${BIBINPUTS} < ${HOME}/prp_ans-1.0/prp_ans.tex > prp_ans.html
scp prp_ans.html dust.ess.uci.edu:/var/www/html/prp/prp_ans-1.0
# NB: tex4ht works well on prp_ans.tex
cd ${HOME}/prp_ans-1.0;htlatex prp_ans.tex
scp prp_ans*.css prp_ans*.html dust.ess.uci.edu:/var/www/html/prp/prp_ans-1.0
# NB: tex4moz works well on prp_ans.tex
cd ${HOME}/prp_ans-1.0;/usr/share/tex4ht/mzlatex prp_ans.tex
scp prp_ans*.css prp_ans*.html prp_ans*.xml dust.ess.uci.edu:/var/www/html/prp/prp_ans-1.0

# Proposal preparation: 
# Divvy up master PDF into FastLane components
pdftk A=${DATA}/ps/prp_ans.pdf cat A3 output ${DATA}/prp/prp_ans/prp_ans_smr.pdf
pdftk A=${DATA}/ps/prp_ans.pdf cat A4-18 output ${DATA}/prp/prp_ans/prp_ans_dsc.pdf
pdftk A=${DATA}/ps/prp_ans.pdf cat A19-23 output ${DATA}/prp/prp_ans/prp_ans_rfr.pdf
pdftk A=${DATA}/ps/prp_ans.pdf cat A24-26 output ${DATA}/prp/prp_ans/prp_ans_bdg_jst.pdf
pdftk A=${DATA}/ps/prp_ans.pdf cat A27 output ${DATA}/prp/prp_ans/prp_ans_fcl.pdf
pdftk A=${DATA}/ps/prp_ans.pdf cat A28-29 output ${DATA}/prp/prp_ans/prp_ans_abb.pdf
pdftk A=${DATA}/ps/prp_ans.pdf cat A30 output ${DATA}/prp/prp_ans/prp_ans_clb.pdf

# Add letters of support in one command rather than loop
# pdftk does not allow input file to be output file
pdftk A=${DATA}/prp/prp_ans/prp_ans_ltr_warren.pdf \
B=${DATA}/prp/prp_ans/prp_ans_ltr_lanl.pdf \
C=${DATA}/prp/prp_ans/prp_ans_ltr_mahowald.pdf \
D=${DATA}/prp/prp_ans/prp_ans_ltr_polarcat.pdf \
cat A B C D output ${DATA}/prp/prp_ans/prp_ans_ltr.pdf

# Add supplementary files in one command rather than loop
# pdftk does not allow input file to be output file
pdftk A=${DATA}/ps/prp_ans.pdf \
B=${DATA}/prp/prp_ans/prp_ans_ltr.pdf \
C=${DATA}/prp/prp_ans/prp_ans_cv_zender.pdf \
D=${DATA}/prp/prp_ans/prp_ans_cp_zender.pdf \
cat A B C D output ${DATA}/ps/prp_ans_fll.pdf
} % end csznote on usage

\end{document}
